Generally speaking, from my own opinion supplements are not necessary on a properly balanced Raw Paleo diet.
If you were depleted of nutrients before going raw paleo you can correct the deficiency with diet alone.
Just eat the whole animal, along with a variety of plant foods that best suit your needs.
Eat bone marrow, organs, blood, glands, fats, etc. If you feel like you need iodine eat a raw thyroid gland from a clean pasture raised animal, or pig out on some raw sea food.